典型文献
Direct conversion of N2 and O2:status,challenge and perspective
文献摘要：
As key components of air,nitrogen(N2)and oxygen(O2)are the vital constituents of lives.Synthesis of NO2,and C-N-O organics direct from N2 and O2,rather than from an intermediate NH3(known as the Haber-Bosch process),is tantalizing.However,the extremely strong N≡N triple bond(945 kJ mol-1)and the nonpolar stable electron configuration of dinitrogen lead to its conversion being extensively energy demanding.The further selective synthesis of high-value C-N-O organics directly from N2,O2 and C-containing molecules is attractive yet greatly challenging from both scientific and engineering perspectives.Enormous efforts have been dedicated to the direct conversion of N2 and O2 via traditional and novel techniques,including thermochemical,plasma,electrochemical,ultrasonic and photochemical conversion.In this review,we aim to provide a thorough comprehension of the status and challenge of the direct conversion of N2,O2 and C-containing molecules(particularly N2 and O2).Moreover,we will propose some future perspectives to stimulate more inspiration from the scientific community to tackle the scientific and engineering challenges.
文献关键词：
中图分类号：
作者姓名：
Di Li;Lingxing Zan;Shiming Chen;Zhang-Jie Shi;Ping Chen;Zhenfeng Xi;Dehui Deng
作者机构：
State Key Laboratory of Catalysis,Collaborative Innovation Center of Chemistry for Energy Materials,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China;Department of Chemistry,Fudan University,Shanghai 200433,China;Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China;Beijing National Laboratory for Molecular Sciences(BNLMS)Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of Education,College of Chemistry,Peking University,Beijing 100871,China
文献出处：
引用格式：
[1]Di Li;Lingxing Zan;Shiming Chen;Zhang-Jie Shi;Ping Chen;Zhenfeng Xi;Dehui Deng-.Direct conversion of N2 and O2:status,challenge and perspective)[J].国家科学评论（英文版）,2022(12):221-237
A类：
tantalizing
B类：
Direct,conversion,N2,status,key,components,air,oxygen,are,vital,constituents,lives,Synthesis,NO2,organics,from,rather,than,intermediate,NH3,known,Haber,Bosch,process,However,extremely,strong,triple,bond,kJ,nonpolar,stable,electron,configuration,dinitrogen,lead,its,being,extensively,energy,demanding,further,selective,synthesis,high,value,directly,containing,molecules,attractive,yet,greatly,challenging,both,scientific,engineering,perspectives,Enormous,efforts,have,been,dedicated,via,traditional,novel,techniques,including,thermochemical,plasma,electrochemical,ultrasonic,photochemical,In,this,review,aim,provide,thorough,comprehension,particularly,Moreover,will,propose,some,future,stimulate,more,inspiration,community,tackle,challenges
AB值：
0.633603
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